Quantum simulators promise to offer new insights into strongly correlated matter beyond what is accessible by means of classical computers. We propose dynamical quantum simulators (DQSs) as a method to simulate dynamical structure factors (DSFs) for system sizes considerably larger than what classical simulations can compute and provide complexity-theoretic evidence that they cannot be classically efficiently computed. Based on state-of-the-art experimental setups, we show how results from DQSs can be directly compared to experiments exploring properties of quantum materials. At the same time, we explore long-ranged spin systems: In particular, we show that the DSFs in DQSs can exhibit the signatures of excitation confinement in long-ranged models for which a comprehensive understanding is lacking. This work has been published in the Proceedings of the National Academy of Sciences (PNAS). A press release can be found here.